Most greatest hits albums tag the metadata for each song with the original album name. You may not have the album, per say, but you do have a piece of it.
I don't see any folder view for the TouchSmart software, only album, artist, genre, etc.
Browsing by artist may be a decent workaround, but if you want to use album, all you should need to do is edit the metadata for your greatest hits albums, and change the album name for each song to "Greatest hits" or something similar. You can do this in Windows Media Player, and you can re-tag all songs in the same album at once.
Mind Over Matt'er - Technology musings, opinion, and more straight from TechLore's head geek.
RSS

